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Picosecond energy transfer in quantum dot Langmuir-Blodgett nanoassemblies

Article Abstract:

The spectrally resolved dynamics of Forster energy transfer (ET) in single monolayers and bilayers of semiconductor nanocrystal quantum dots assembled (CdSe NQDs) fabricated using Langmuir-Blodgett (LB) techniques are studied. By analyzing spectrally resolved photoluminescence (PL) dynamics, it was found that ET is dominated by interactions of a center, donor NQD with NQD acceptors from the first three shells; as a result, the ET-related PL dynamics can be fit by a sum of three exponential decay terms in which each term is associated with a specific shell

Author: Klimov, Victor I., Achermann, Marc, Petruska, Melissa A., Crooker, Scott A.
Publisher: American Chemical Society
Publication Name: Journal of Physical Chemistry B
Subject: Chemicals, plastics and rubber industries
ISSN: 1520-6106
Year: 2003
Thin films, Multilayered, Multilayered thin films, Energy transfer, Photoluminescence

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Light amplification using inverted core/shell nanocrystals: towards lasing in the single-exciton regime

Article Abstract:

A novel approach to achieve NC lasing in the Auger-recombination-free regime by using type II NC heterostructures that promote spatial separation on electrons and holes is explored. It is presented that such hetero-NCs can exhibit strong repulsive excition-excition interactions that lead significantly reduced excited-state absorption associated with NCs containing single electron-hole pairs.

Author: Klimov, Victor I., Tretiak, Sergei, Achermann, Marc, Ivanov, Sergei A., Nanda, Jagjit, Piryatinski, Andrei, Balet, Laurent P,, Bezel, Ilia V, Anikeeva, Polina O.
Publisher: American Chemical Society
Publication Name: Journal of Physical Chemistry B
Subject: Chemicals, plastics and rubber industries
ISSN: 1520-6106
Year: 2004
Optical properties, Electrons, Excited state chemistry

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Inter-specific vibrational spectroscopy of molecules with visible lights

Article Abstract:

A more general solution, a time-domain spectroscopy based on fourth-order Raman scattering in which vibrational coherences are pumped by a Raman process is proposed. Fourier transformation of the oscillation provides a vibrational spectrum of 0-1000 cm(super -1) for the dye located at the ir-solution interface.

Author: Klimov, Victor I., Tretiak, Sergei, Ishibashi, Taka-aki, Onishi, Hiroshi, Achermann, Marc, Fujiyoshi, Satoru, Anikeeva, Polina O., Bezel, Ilia V., Balet, Laurent P
Publisher: American Chemical Society
Publication Name: Journal of Physical Chemistry B
Subject: Chemicals, plastics and rubber industries
ISSN: 1520-6106
Year: 2004
Fourier transform infrared spectroscopy, Raman effect, Vibrational spectra

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Subjects list: Research, Usage, Chemistry, Physical and theoretical, Physical chemistry, Observations
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